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Physical Chemistry Chemical Physics 2009, 11 A volcano curve: optimizing methanol electro-oxidation on Pt-decorated Ru nanoparticles. Rabb, Christopher Zangmeister, YuYe Tong. Journal of Applied Electrochemistry 2009, 39 Electro-reduction of oxygen and electro-oxidation of methanol at Pd monolayer-modified macroporous Pt electrode. Yongling Du, Kangle Lv, Biquan Su, Nuo Zhang, Chunming Wang.Methanol and formic acid oxidation on ad-metal modified electrodes. Methanol electrooxidation at mesoporous Pt and PtвЂ“Ru electrodes: A comparative study with carbon supported materials. Gonzalo GarcГa, Jonathan Florez-MontaГ±o, Alberto Hernandez-Creus, Elena Pastor, Gabriel A.Electroanalysis using modified hierarchical nanoporous carbon materials. Rusbel Coneo Rodriguez, Angelica Baena Moncada, Diego F.Effect on CO and methanol electrooxidation. A novel method to produce a hierarchical porous carbon as a conductive support of PtRu particles. Role of Hydrous Ruthenium Oxide in Ptв€’Ru Direct Methanol Fuel Cell Anode Electrocatalysts: The Importance of Mixed Electron/Proton Conductivity. Complexes with Platinumв€’Ruthenium Bonds: The Stepwise Formation of Complexes Containing PtRu and PtRu2 Units.

Complexes with Platinumв€’Ruthenium Bonds: Synthesis, Structure, and Fluxionality of Pt3Ru Cluster Complexes. The Journal of Physical Chemistry B 2000, 104

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How To Make Electrocatalysts More Active for Direct Methanol OxidationAvoid PtRu Bimetallic Alloys!. Surface Coordination of Ruthenium Clusters on Platinum Nanoparticles for Methanol Oxidation Catalysts. The Journal of Physical Chemistry B 2005, 109 Ru-Decorated Pt Surfaces as Model Fuel Cell Electrocatalysts for CO Electrooxidation. The Journal of Physical Chemistry B 2006, 110 Multiwalled Carbon Nanotube Supported PtRu for the Anode of Direct Methanol Fuel Cells. High-Throughput Synthesis and Screening of Ternary Metal Alloys for Electrocatalysis. Nanostructure PtRu/MWNTs as Anode Catalysts Prepared in a Vacuum for Direct Methanol Oxidation. PtRu Nanoparticle Electrocatalyst with Bulk Alloy Properties Prepared through a Sonochemical Method.

Rukma Basnayake, Zhengrong Li, Srilakshmi Katar, Wei Zhou, Harry Rivera, Eugene S.

Ethylene Substitution in a Bis-Ethylene Complex of Rh/Os and Unusual BrГёnstedв€’Lowry Basicity of an N-Heterocyclic Carbene. Ferguson, Robert McDonald, and Martin Cowie. The Journal of Physical Chemistry C 2015, 119 Second Order Dependence on the Surface Fraction of Pt in Pt-Ruadatom of the Oxidation of 2-PrOH in Base. This article is cited by 41 publications. The activation energies for oxidation of MeOH over 0.05 and 0.10 equiv of Ptв€’Ru ad were 37 and 45 kJ/mol, respectively, at 0.4 V, 0.5 M H 2SO 4, and 0.5 M MeOH. Surfaces with low equivalents of Ru adatoms (from 0.05 to 0.10 equiv) were the most active toward the potentiostatic oxidation of MeOH ( E = 0.4 V, 0.5 M H 2SO 4, 0.5 M MeOH, 25 вЊ) with between 50 and 28 times higher turnover numbers than black Pt. The activity of Pt increased relative to the other surfaces as the potential increased, becoming more active than 0.30, 0.70, and 0.44 equiv Ptв€’Ru ad at the upper limit of the sweeps. The order of activity of MeOH-poisoned Ptв€’Ru ad surfaces toward the potentiodynamic oxidation of MeOH (0.5 M H 2SO 4, 25 вЊ, sweep range 0.025в€’0.60 V, 5 mV/s) was 0.05 > 0.10 > 0.30 в€ј 0.44 > 0.7 > 0 (Pt) equiv of Ru adatoms. The measured currents were normalized to the specific surface areas of the gauzes measured before deposition of Ru adatoms by hydrogenation of 1. The surfaces were evaluated as catalysts for the electrooxidation of MeOH. Deposition of more Ru adatoms did not cause significant further drops in the CO stripping peak potential. Stripping voltammetry of adsorbed monolayers of carbon monoxide from these surfaces (0.5 M H 2SO 4, 25 вЊ, sweep range 0.025в€’0.70 V, 5 mV/s) showed a drop by 120 mV in the CO stripping peak potential upon deposition of 0.05 equiv of Ru adatoms on Pt. The ratio of currents in the вЂњdouble layerвЂќ to those in the вЂњhydrideвЂќ region in the potentiodynamic responses of these surfaces (0.5 M H 2SO 4, 25 вЊ, sweep range 0.025в€’0.70 V, 5 mV/s) increased as the equivalents of Ru adatoms increased.

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A series of Ptв€’Ru ad surfaces were prepared by interrupting the hydrogenation after deposition of 0.05, 0.10, 0.30, 0.32, 0.44, 0.70, and 3.5 equiv of Ru adatoms. Ru adatoms were deposited on black Pt gauze by hydrogenating Ru(COD)(О· 3-C 3H 5) 2 ( 1, COD is 1,5-cyclooctadiene) over the gauze at low temperatures in hexanes solution under 1 atm of dihydrogen gas.

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